Science & Technology Complex
The mixture of techniques indicated that U uptake is split into three-phases; initial adsorption of U(VI), reduction of U(VI) to UO nanoprecipitates at surface-particular sites after 2-3 h of publicity, and completion of U(VI) reduction after ~6-eight h. U(VI) discount additionally corresponded to detectable will increase in Fe launched to answer and surface topography changes.
Sci-tech 1-019
Redox reactions are proposed that explicitly couple the discount of U(VI) to enhanced release of Fe(II) from magnetite. Although counterintuitive, the proposed reaction stoichiometry was proven to be largely according to the experimental outcomes. In addition to providing molecular-scale particulars about U sorption on magnetite, this work additionally presents novel advances for collecting surface delicate molecular-scale info in real-time under batch-circulate conditions.
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